TPV Research: Nonlinear Polymer Behavior

Fig. Macro-scale version of TPV microstructure, particle in matrix

The Problem

TPV (Thermoplastic Vulcanizates) is a high-performance rubber-plastic polymer widely used in seals, gaskets, and weather strips.

However, the relationship between its microstructure and mechanical behavior is not well understood, particularly the deformation mechanisms. This project was set to investigate how the spatial arrangement of particles within the stiff matrix drives local deformation mechanisms.

To study this, I needed a repeatable, controlled way to fabricate and test samples of TPV.

Fig. 3D STEP files for Polyjet Printing

The Approach

Geometry Generation Pipeline

  • Developed a Python script to parametrically generate periodic samples with tunable parameters: volume fraction, particle size, arrangement, and randomness

  • Generated 8 unique patterns

  • Exported multi-material STEP files for direct PolyJet 3D printing

Fig. Plane-strain compression fixture

Fixture Design

  • Designed and fabricated a custom plane-strain compression fixture

  • Modeled custom 3D printed parts, laser-cut acrylic platens, and ordered custom steel standoffs

Fig. Plane-strain compression fixture

Physical Testing

  • Tested 12 specimens on a Zwick-Roell universal testing machine to 20% compressive strain

  • Tested specimens in multiple loading orientations to probe anisotropy

  • Conducted post processing and data analysis

The Result & Impact

  • Showed particle arrangement drives stiffness more than size distribution.

    • Single-grid packing was ~2.5× stiffer than staggered at identical volume fraction

  • Demonstrated that scaling particles down 0.5× at constant Vf increases stiffness and reduces anisotropy

  • Built a fully reusable geometry pipeline extensible to elliptical and rectangular particle shapes

  • Established that deformation localizes through the thinnest matrix ligaments.

    • Path of least resistance governs local failure across all cases

Full report here: https://docs.google.com/presentation/d/1tqTEQPi9rF2Xm-dwzfrscMXKAoydU9MesYvWJ5Fpe1o/edit?usp=sharing

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